"Tired of Toein' the Line", by Rocky Burnette.
Nah, just kidding. (Though that video is pretty freakin' awesome.)
Actually, it's:
"Come on Home to Me", by Tracey Thorn.
Tracey Thorn. Jens Lekman. Lee Hazlewood. It's a marriage made in heaven. (Sadly, in Lee's case, literally so.) In fact, I assumed it would be too good to be true. And yet it turns out that the song, which is way different from what I expected it to be, is much, much better than it would have been if it had been what I expected it to be. There. That makes complete sense, doesn't it?